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Visualizing single atom dynamics in heterogeneous catalysis using analytical in situ environmental scanning transmission electron microscopy

Boyes, Edward D ; LaGrow, Alec P ; Ward, Michael R ; Martin, Thomas E ; Gai, Pratibha L

Philosophical transactions of the Royal Society of London. Series A: Mathematical, physical, and engineering sciences, 2020-12, Vol.378 (2186), p.20190605-20190605 [Periódico revisado por pares]

England: The Royal Society Publishing

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  • Título:
    Visualizing single atom dynamics in heterogeneous catalysis using analytical in situ environmental scanning transmission electron microscopy
  • Autor: Boyes, Edward D ; LaGrow, Alec P ; Ward, Michael R ; Martin, Thomas E ; Gai, Pratibha L
  • Assuntos: Review
  • É parte de: Philosophical transactions of the Royal Society of London. Series A: Mathematical, physical, and engineering sciences, 2020-12, Vol.378 (2186), p.20190605-20190605
  • Notas: ObjectType-Article-1
    SourceType-Scholarly Journals-1
    ObjectType-Feature-2
    content type line 23
    One contribution of 10 to a discussion meeting issue ‘Dynamic in situ microscopy relating structure and function’.
  • Descrição: Progress is reported in analytical environmental scanning transmission electron microscopy (ESTEM) for visualizing and analysing in real-time dynamic gas-solid catalyst reactions at the single-atom level under controlled reaction conditions of gas environment and temperature. The recent development of the ESTEM advances the capability of the established ETEM with the detection of fundamental single atoms, and the associated atomic structure of selected solid-state heterogeneous catalysts, in catalytic reactions in their working state. The new data provide improved understanding of dynamic atomic processes and reaction mechanisms, in activity and deactivation, at the fundamental level; and in the chemistry underpinning important technological processes. The benefits of atomic resolution-E(S)TEM to science and technology include new knowledge leading to improved technological processes, reductions in energy requirements and better management of environmental waste. This article is part of a discussion meeting issue 'Dynamic microscopy relating structure and function'.
  • Editor: England: The Royal Society Publishing
  • Idioma: Inglês
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