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Tungsten-Based Catalysts for Selective Deoxygenation

Gosselink, Robert W. ; Stellwagen, Daniel R. ; Bitter, Johannes H.

Angewandte Chemie (International ed.), 2013-05, Vol.52 (19), p.5089-5092 [Periódico revisado por pares]

Weinheim: WILEY-VCH Verlag

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  • Título:
    Tungsten-Based Catalysts for Selective Deoxygenation
  • Autor: Gosselink, Robert W. ; Stellwagen, Daniel R. ; Bitter, Johannes H.
  • Assuntos: Atmospheres ; Biobased Chemistry and Technology ; biomass ; Catalysis ; Catalysts ; Decarboxylation ; Deoxygenation ; nanostructures ; olefins ; Pathways ; supported catalysts ; Tungsten ; Tungsten oxides ; Vegetables ; VLAG
  • É parte de: Angewandte Chemie (International ed.), 2013-05, Vol.52 (19), p.5089-5092
  • Notas: ark:/67375/WNG-4B7JX6QH-Z
    Netherlands Ministry of Education, Culture, and Science
    This research has been performed within the framework of the CatchBio program. We gratefully acknowledge the support of the Smart Mix Program of the Netherlands Ministry of Economic Affairs and the Netherlands Ministry of Education, Culture, and Science. Philip Walder is kindly acknowledged for the equipment preparation and initial experiments. We thank Lucian Roiban for the TEM measurements, Jesper Sättler for his help during Raman analysis, and Krijn de Jong for discussions and suggestions.
    istex:25ADF1D5A6ED0878DDCE25D50826E358DB6B28A2
    Netherlands Ministry of Economic Affairs
    ArticleID:ANIE201209809
    These authors contributed equally to this work.
    ObjectType-Article-1
    SourceType-Scholarly Journals-1
    ObjectType-Feature-2
    content type line 23
  • Descrição: On the tip of the tung(sten): The title catalysts selectively perform deoxygenation of vegetable‐oil‐based feeds by either decarboxylation/decarbonylation or hydrodeoxygenation (HDO) pathways, depending on the dominant tungsten phase (WO3 and W2C). The process upgrades vegetable‐oil‐based feeds, under a hydrogen atmosphere, to high‐value olefinic products, thus providing a significant advantage over other types of deoxygenation catalysts.
  • Editor: Weinheim: WILEY-VCH Verlag
  • Idioma: Inglês
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