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New advances in nanographene chemistry
Narita, Akimitsu ; Wang, Xiao-Ye ; Feng, Xinliang ; Müllen, Klaus
Chemical Society reviews, 2015-09, Vol.44 (18), p.6616-6643
[Periódico revisado por pares]
England
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Título:
New advances in nanographene chemistry
Autor:
Narita, Akimitsu
;
Wang, Xiao-Ye
;
Feng, Xinliang
;
Müllen, Klaus
É parte de:
Chemical Society reviews, 2015-09, Vol.44 (18), p.6616-6643
Notas:
Xinliang Feng, after obtaining his Master's degree in organic chemistry from Shanghai Jiao Tong University in March 2004, joined the group of Prof. K. Müllen at the Max Planck Institute for Polymer Research (MPIP) and obtained his PhD in April 2008. He became a group leader at MPIP in December 2007. Since June 2010, he has been a professor at Shanghai Jiao Tong University and became a distinguished group leader at MPIP in 2012. In August 2014, he became a chair professor at Dresden University of Technology. His current scientific interests include graphene, two-dimensional nanomaterials, organic conjugated materials, and carbon-rich molecules and materials for electronic and energy-related applications.
Klaus Müllen received his PhD in 1972 at the University of Basel (Professor F. Garson) after completing his Diploma in Chemistry at the University of Cologne (Professor E. Vogel) in 1969. He pursued postdoctoral research in the group of J. F. M. Oth at ETH Zurich, where he received his habilitation in 1977 and was appointed a Privatdozent. In 1979, he became a Professor in Organic Chemistry at the University of Cologne and accepted an offer of a chair in Organic Chemistry at the University of Mainz in 1983. In 1989, he became a scientific member of the Max Planck Society and has been the director of the Synthetic Chemistry Department at the Max Planck Institute for Polymer Research. He served as President of the German Chemical Society for two years, beginning January 2008. His current research focuses on synthetic macromolecular chemistry, supramolecular chemistry, and materials science.
Akimitsu Narita was born in Yokohama, Japan in 1986. He received his Bachelor's (2008) and Master's (2010) degrees in Chemistry at the University of Tokyo under the supervision of Professor Eiichi Nakamura. In March 2014, he obtained his PhD in the group of Professor Klaus Müllen at the Max Planck Institute for Polymer Research (MPIP) in Mainz. He was an Early-Stage Researcher in the Marie-Curie Initial Training Network (ITN) "SUPERIOR" for three years from May 2010. Beginning in August 2014, he became a project leader in the Synthetic Chemistry Department at MPIP. His current research focuses on the bottom-up organic synthesis of functional graphene molecules and graphene nanoribbons.
Xiao-Ye Wang was born in China in 1989. He received his Bachelor's degree in chemistry from Nankai University in 2009. In the same year, he joined Professor Jian Pei's group at Peking University as a graduate student and obtained his PhD degree in organic materials chemistry in July 2014. Then he joined the group of Professor Klaus Müllen at the Max Planck Institute for Polymer Research (MPIP) for postdoctoral research. His research interests include organic electronic materials and devices as well as bottom-up synthesis of heteroatom-doped graphene molecules and graphene nanoribbons.
ObjectType-Article-1
SourceType-Scholarly Journals-1
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content type line 23
Descrição:
Nanographenes, or extended polycyclic aromatic hydrocarbons, have been attracting renewed and more widespread attention since the first experimental demonstration of graphene in 2004. However, the atomically precise fabrication of nanographenes has thus far been achieved only through synthetic organic chemistry. The precise synthesis of quasi-zero-dimensional nanographenes, i.e. graphene molecules, has witnessed rapid developments over the past few years, and these developments can be summarized in four categories: (1) non-conventional methods, (2) structures incorporating seven- or eight-membered rings, (3) selective heteroatom doping, and (4) direct edge functionalization. On the other hand, one-dimensional extension of the graphene molecules leads to the formation of graphene nanoribbons (GNRs) with high aspect ratios. The synthesis of structurally well-defined GNRs has been achieved by extending nanographene synthesis to longitudinally extended polymeric systems. Access to GNRs thus becomes possible through the solution-mediated or surface-assisted cyclodehydrogenation, or "graphitization," of tailor-made polyphenylene precursors. In this review, we describe recent progress in the "bottom-up" chemical syntheses of structurally well-defined nanographenes, namely graphene molecules and GNRs. This review discusses recent advancements in nanographene chemistry, focusing on the bottom-up synthesis of graphene molecules and graphene nanoribbons.
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England
Idioma:
Inglês
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