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Transition‐Metal‐Catalyzed Selective Functionalization of C(sp3)−H Bonds in Natural Products

Karimov, Rashad R. ; Hartwig, John F.

Angewandte Chemie (International ed.), 2018-04, Vol.57 (16), p.4234-4241 [Periódico revisado por pares]

Germany: Wiley Subscription Services, Inc

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  • Título:
    Transition‐Metal‐Catalyzed Selective Functionalization of C(sp3)−H Bonds in Natural Products
  • Autor: Karimov, Rashad R. ; Hartwig, John F.
  • Assuntos: amination ; Biological Products - chemical synthesis ; Biological Products - chemistry ; Catalysis ; Chemical bonds ; C−H bond functionalization ; Metals ; Molecular Conformation ; Molecular structure ; Natural products ; oxidation ; regioselectivity ; Transition Elements - chemistry
  • É parte de: Angewandte Chemie (International ed.), 2018-04, Vol.57 (16), p.4234-4241
  • Notas: ObjectType-Article-1
    SourceType-Scholarly Journals-1
    ObjectType-Feature-3
    content type line 23
    ObjectType-Review-2
  • Descrição: Direct functionalization of natural products is important for studying the structure–activity and structure–property relationships of these molecules. Recent advances in the transition‐metal‐catalyzed functionalization of C(sp3)−H bonds, the most abundant yet inert bonds in natural products, have allowed natural product derivatives to be created selectively. Strategies to achieve such transformation are reviewed. Direct derivatization: Direct functionalization of natural products is important for studying their structure–activity and structure–property relationships. Recent advances in the transition‐metal‐catalyzed functionalization of C(sp3)−H bonds have shown that natural product derivatives can be selectively produced. Strategies for achieving such transformations are discussed.
  • Editor: Germany: Wiley Subscription Services, Inc
  • Idioma: Inglês
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