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Elektrochemische Carborankäfig‐Aktivierung
Yang, Long ; Zhang, Zi‐Jing ; Bongsuiru Jei, Becky ; Ackermann, Lutz
Angewandte Chemie, 2022-05, Vol.134 (20), p.n/a
[Peer Reviewed Journal]
Weinheim: Wiley Subscription Services, Inc
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Title:
Elektrochemische Carborankäfig‐Aktivierung
Author:
Yang, Long
;
Zhang, Zi‐Jing
;
Bongsuiru Jei, Becky
;
Ackermann, Lutz
Subjects:
Carborane
;
Chemistry
Is Part Of:
Angewandte Chemie, 2022-05, Vol.134 (20), p.n/a
Description:
Carborane sind Bor‐Kohlenstoff‐Molekülcluster, welche einzigartige Eigenschaften aufweisen, wie ihre ikosaedrische Geometrie, einen hohen Bor‐Anteil und eine dreidimensional delokalisierte Aromatizität. Diese machen Carborane zu wertvollen Bausteinen in verschiedenen Anwendungsbereichen, wie supramolekularem Design, Nanomaterialien, Optoelektronik, Bor‐Neutroneneinfangtherapeutika (BNCT) und metallorganischer sowie Koordinationschemie. Trotz weitreichender Fortschritte auf diesem Forschungsgebiet werden stöchiometrische Mengen chemischer Redox‐Reagenzien weiterhin für die oxidative Aktivierung der Carborankäfige benötigt. In diesem Kontext ist die elektrochemische Synthese eine vielversprechende und nachhaltige Alternative. In den vergangenen Jahren konnte erheblicher Fortschritt in der elektrochemischen Käfig‐Funktionalisierung an Carboranen erzielt werden, welcher hier zusammengefasst wurde. Wir erwarten, dass die Elektrokatalyse innerhalb der aktuellen Renaissance der Carboran‐Elektrochemie einen immer stärkeren Impuls geben wird. Trotz einer Renaissance der Carborankäfig‐Aktivierung in den letzten Jahrzehnten erfordern oxidative Käfigfunktionalisierungen im Allgemeinen stöchiometrische Mengen an toxischen chemischen Oxidationsmitteln. Im Gegensatz dazu ermöglichen elektrochemische Funktionalisierungen eine ressourcenschonende Käfigaktivierung.
Publisher:
Weinheim: Wiley Subscription Services, Inc
Language:
English
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